光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
EPS={w$'s !xP8#|1 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
ZaeqOVp/j ;w'D4p= P 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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'cx_F K3m]%m2\ 目录
g) p,5BADm 1. Introduction and Basic Principles
(:._"jp] 1.1 Historical Development
io,M{Ib 1.2 The Electron Mean Free Path
T6H}/#*tK 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
U"q/rcA 1.4 Experimental Aspects
A:aE|v/T& 1.5 Very High Resolution
S>.SSXlM 1.6 The Theory of Photoemission
V2$h8\a 1.6.1 Core-Level Photoemission
s4 6}s{6 1.6.2 Valence-State Photoemission
qY~`8
x 1.6.3 Three-Step and One-Step Considerations
L !=4N!j 1.7 Deviations from the Simple Theory of Photoemission
QA2borfy References
Sl-v W Jj,U RD&0R 2. Core Levels and Final States
d*A*y ^OD 2.1 Core-Level Binding Energies in Atoms and Molecules
.uyGYj-C 2.1.1 The Equivalent-Core Approximation
?"zY"*>4 2.1.2 Chemical Shifts
t<~ $ 2.2 Core-Level Binding Energies in Solids
6fd+Q
/ 2.2.1 The Born-Haber Cycle in Insulators
v3}L`dyh3 2.2.2 Theory of Binding Energies
vJ\pR~? 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
}| J79s2M 2.3 Core Polarization
70f Klp 2.4 Final-State Multiplets in Rare-Earth Valence Bands
r) $+ 2.5 Vibrational Side Bands
2kdC]|H2? 2.6 Core Levels of Adsorbed Molecules
L,mQ
2.7 Quantitative Chemical Analysis from Core-Level Intensities
IB#
@yH References
p!sWYui pX&pLaF 3. Charge-Excitation Final States: Satellites
!PrwH; 3.1 Copper Dihalides; 3d Transition Metal Compounds
o4*+T8[|5 3.1.1 Characterization of a Satellite
0G7K8`a 3.1.2 Analysis of Charge-Transfer Satellites
XK|R8rhg8` 3.1.3 Non-local Screening
1WY/6[ 3.2 The 6-eV Satellite in Nickel
tjGd ) 3.2.1 Resonance Photoemission
Kl2lbe7 3.2.2 Satellites in Other Metals
2 Yp7 3.3 The Gunnarsson-Sch6nhammer Theory
K?s+ 3 3.4 Photoemission Signals and Narrow Bands in Metals
T/^Hz4uA7 References
MF~H"D
n qHNE8\9 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
w"OP8KA:^T 4.1 Theory
pY_s*0_ 4.1.1 General
e*bH0'; q 4.1.2 Core-Line Shape
Kw8u`$Ad7 4.1.3 Intrinsic Plasmons
R,9[hNHWGs 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
3 n'V\Hvz 4.1.5 The Total Photoelectron Spectrum
F)s{P Cl 4.2 Experimental Results
Ix(?fO#uNF 4.2.1 The Core Line Without Plasmons
N@Y ljz| 4.2.2 Core-Level Spectra Including Plasmoas
io#&o;M< 4.2.3 Valence-Band Spectra of the Simple Metals
{"&SJt[%X 4.2.4 Simple Metals: A General Comment
JJ{9U(`_y6 4.3 The Background Correction
|N}P(GF References
s3]?8hXd C?i >.t 5. Valence Orbitals in Simple Molecules and Insulating Solids
d}JP!xf% 5.1 UPS Spectra of Monatomic Gases
K4]g[z 5.2 Photoelectron Spectra of Diatomic Molecules
bYi`R) 5.3 Binding Energy of the H2 Molecule
YO}1(m 5.4 Hydrides Isoelectronic with Noble Gases
hGbj0 Neon (Ne)
:6zG7qES3 Hydrogen Fluoride (HF)
AX= 1b,s Water (H2O)
4O;OjUI0a Ammonia (NH3)
mt5KbA>nU Methane (CH4)
M/):e$S 5.5 Spectra of the Alkali HMides
ep=qf/vd< 5.6 Transition Metal Dihalides
34wkzu 5.7 Hydrocarbons
wE@'ap# 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
n>A98NQ 5.7.2 Linear Polymers
[5uRS}! 5.8 Insulating Solids with Valence d Electrons
[@Q_(LQ-U 5.8.1 The NiO Problem
7zHh@ B:] 5.8.2 Mort Insulation
]S(%[| 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
-i4&v7" 5.8.4Band Structures of Transition Metal Compounds
7ULqo>j 5.9 High—Temperature Superconductors
yv\#8I:qh 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
Ux#x#N 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
e|&6$A>4] 5.9.3 The Superconducting Gap
]~6_ WE8L 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
C_4)=#@GU 5.9.5 Core—Level Shifts
@BrMl%gV 5.10 The Fermi Liquid and the Luttinger Liquid
T"&)&"W*U 5.11 Adsorbed Molecules
:.?gHF.? 5.11.1 Outline
yuDZ~0]R 5.11.2 CO on Metal Surfaces
?{U
m References
o99pHW(E rp6q?3=g 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
zH>hx5,k'X 6.1 Theory of Photoemission:A Summary of the Three-Step Model
MY/3]g< 6.2 Discussion of the Photocurrent
!!4Qj 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
Kh4$ wwn 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
(`6T&>(4 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
K{ \;2M 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
P%#*-zCCx 6.3.1 Band Structure Regime
lj{VL}R 6.3.2 XPS Regime
p/2jh& 6.3.3 Surface Emission
GEEW?8 6.3.4 One-Step Calculations
j:}D Bk 6.4 Thermal Effects
0]D{Va 6.5 Dipole Selection Rules for Direct Optical Transitions
=)E,8L References
&z]K\-xp =7m}yDs6$ 7.Band Structtire and Angular-Resolved Photoelectron Spectra
quvanxV-L 7.1 Free-Electron Final—State Model
@ JvPx 0 7.2 Methods Employing Calculated Band Structures
;L|uIg;.s 7.3 Methods for the Absolute Determination of the Crystal Momentum
?7M.o 7.3.1 Triangulation or Energy Coincidence Method
0<8XI>.3D 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
r}0\}~'?c 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
v^ /Q 8Q 7.3.4 The Surface Emission Method and Electron Damping
[kqYfY?K 7.3.5 The Very-Low-Energy Electron Diffraction Method
:>aQ~1f>] 7.3.6 The Fermi Surface Method
<\0vR20/ 7.3.7 Intensities and Their Use in Band-Structure Determinations
R(-<BtM!- 7.3.8 Summary
gJ;_$` 7.4 Experimental Band Structures
.`7cBsXH 7.4.1 One- and Two-Dimensional Systems
K"uNxZ 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
McoK@q; 7..4.3UPS Band Structures and XPS Density of States
rJa$9B*^ 7.5 A Comment
(ZL sB{r^ References
7},)]da>,' 557(EM
8.Surface States, Surface Effects
U~W?s(Cy% 8.1 Theoretical Considerations
`+t.!tv! 8.2 Experimental Results on Surface States
[w\9as/ E 8.3 Quantum-Well States
U `o^mtW. 8.4 Surface Core-Level Shifts
(;%|-{7e- References
:K
~ PlYm& 9.Inverse Photoelectron Spectroscopy
-!0_:m3 9.1 Surface States
0<PR+Iv*i 9.2 Bulk Band Structures
>|6iR%"f# 9.3 Adsorbed Molecules
f30Pi1/h=c References
n!6Z]\8~$ be e5 10. Spin-Polarized Photoelectron Spectroscopy
lNv".Y=l 10.1 General Description
[ >^PRs 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
$5L0.$Tj 10.3 Magnetic Dichroism
lCF`*DM# References
1xU3#b&2tC ^'p|!`: 11. Photoelectron Diffraction
+[J/Zw0{ 11.1 Examples
g~BoFc.V2~ 11.2 Substrate Photoelectron Diffraction
Qu<Bu)` 11.3 Adsorbate Photoelectron Diffraction
aF|d^ 11.4 Fermi Surface Scans
<xJ/y|{ References
)HD`O~M> M7>(hVEAW' Appendix
-`f04_@>d A.1 Table of Binding Energies
*_ +7ni A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
)RYG% A.3 Compilation of Work Functions
$
n,Z References
<`!PCuR Index