光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
{W' 9k x :? EL)( 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
XU*4MU^' v =]!Po&Q- 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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o$vI~U, -+HD5Hc 目录
lJJ`aYDp 1. Introduction and Basic Principles
7L4~yazmK 1.1 Historical Development
/D>G4PP< 1.2 The Electron Mean Free Path
lc(}[Z/|V 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
WNK)IC~c 1.4 Experimental Aspects
haSC[[o= 1.5 Very High Resolution
G_E \p%L>] 1.6 The Theory of Photoemission
PNB E 1.6.1 Core-Level Photoemission
<HfmNhI85( 1.6.2 Valence-State Photoemission
U3^3nL-M9 1.6.3 Three-Step and One-Step Considerations
8#ZF<BY 1.7 Deviations from the Simple Theory of Photoemission
(`js/7[`H[ References
IJk<1T7:(W
'E)g )@^ 2. Core Levels and Final States
>9+h2B
2.1 Core-Level Binding Energies in Atoms and Molecules
vUR@P
- 2.1.1 The Equivalent-Core Approximation
-%ftPfm 2.1.2 Chemical Shifts
c\.7Z=D 2.2 Core-Level Binding Energies in Solids
.FeVbZW 2.2.1 The Born-Haber Cycle in Insulators
DEQ7u`6 2.2.2 Theory of Binding Energies
6R|^IPOGp 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
8zrLl:{ 2.3 Core Polarization
J,D^fVIw 2.4 Final-State Multiplets in Rare-Earth Valence Bands
1a
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r:U/a=V 2.6 Core Levels of Adsorbed Molecules
$)Ty@@7C 2.7 Quantitative Chemical Analysis from Core-Level Intensities
'pHxO,vo References
pn p)- a*7 h#}'9oA 3. Charge-Excitation Final States: Satellites
/2x@Z> 3.1 Copper Dihalides; 3d Transition Metal Compounds
]T; 3.1.1 Characterization of a Satellite
PlRcrT"#w 3.1.2 Analysis of Charge-Transfer Satellites
k9!euj& 3.1.3 Non-local Screening
h'"~t#r 3.2 The 6-eV Satellite in Nickel
>c=-uI 3.2.1 Resonance Photoemission
%fIYWu`X 3.2.2 Satellites in Other Metals
=Bos>;dl 3.3 The Gunnarsson-Sch6nhammer Theory
P{2j31u` 3.4 Photoemission Signals and Narrow Bands in Metals
.W51Cup@& References
&R,QJ4L PB;j4 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
'Gqo{wl 4.1 Theory
H+5S )r 4.1.1 General
* zc[t 4.1.2 Core-Line Shape
OjurfVw 4.1.3 Intrinsic Plasmons
@;7Ht Z` 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
_BI[F
m 4.1.5 The Total Photoelectron Spectrum
IqCh4y3 4.2 Experimental Results
Ns$,.D 4.2.1 The Core Line Without Plasmons
l9z{pZ\KM 4.2.2 Core-Level Spectra Including Plasmoas
Wrf+5 ;,, 4.2.3 Valence-Band Spectra of the Simple Metals
qZ%0p*P#_ 4.2.4 Simple Metals: A General Comment
5Bp>*MR/". 4.3 The Background Correction
|&_(I References
'iX y?l 3oMa 5. Valence Orbitals in Simple Molecules and Insulating Solids
SedVp cb+ 5.1 UPS Spectra of Monatomic Gases
V)c.AX5 5.2 Photoelectron Spectra of Diatomic Molecules
Qov*xRO6 5.3 Binding Energy of the H2 Molecule
%+oV-o\ #A 5.4 Hydrides Isoelectronic with Noble Gases
XB<Q A>dLh Neon (Ne)
T U^s!Tj Hydrogen Fluoride (HF)
<_yy0G Water (H2O)
*})Np0k Ammonia (NH3)
GI%9Tif Methane (CH4)
qT^0
%O: 5.5 Spectra of the Alkali HMides
BeFXC5-qat 5.6 Transition Metal Dihalides
_xGC0f ( 5.7 Hydrocarbons
:8U@KABH@h 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
xTy)qN]P 5.7.2 Linear Polymers
= ,c!V 5.8 Insulating Solids with Valence d Electrons
xiO10:L4 5.8.1 The NiO Problem
Q6r7UM 5.8.2 Mort Insulation
Yb?(Q% 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
LJOJ2x 5.8.4Band Structures of Transition Metal Compounds
]Cp`qayct 5.9 High—Temperature Superconductors
kudXwj 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
I^m9(L4% 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
q>m[vvt" 5.9.3 The Superconducting Gap
m0N{%Mf- 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
7Mb-v} 5.9.5 Core—Level Shifts
sOm&7A? 5.10 The Fermi Liquid and the Luttinger Liquid
,"f2-KC4h 5.11 Adsorbed Molecules
!=?Q>mz 5.11.1 Outline
Bp/25jy 5.11.2 CO on Metal Surfaces
OBf$0 References
m}]\ ^$d \J6&Z13Q 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
$*C'{&2 6.1 Theory of Photoemission:A Summary of the Three-Step Model
IJBIO>Z/ 6.2 Discussion of the Photocurrent
?I7%ueFY 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
.50ql[En 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
pDt45 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
vP^V3 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
=QhK|C!$A 6.3.1 Band Structure Regime
Jp(CBCG{F 6.3.2 XPS Regime
c\VD8 : 6.3.3 Surface Emission
k< 6.3.4 One-Step Calculations
]~9YRVeC 6.4 Thermal Effects
oG=4&SQ 6.5 Dipole Selection Rules for Direct Optical Transitions
Is>~ P*2Y= References
R_Uy.0=4 Na<);Pg 7.Band Structtire and Angular-Resolved Photoelectron Spectra
i}v3MO\X 7.1 Free-Electron Final—State Model
V"8w:? 7.2 Methods Employing Calculated Band Structures
-_irkpdC[ 7.3 Methods for the Absolute Determination of the Crystal Momentum
%18%T{|$e 7.3.1 Triangulation or Energy Coincidence Method
vOU9[n
N[ 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
b5W(}ka+ 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
zE?@_p1gei 7.3.4 The Surface Emission Method and Electron Damping
a7"Aq:IjU 7.3.5 The Very-Low-Energy Electron Diffraction Method
8UXtIuQ 7.3.6 The Fermi Surface Method
\I 7,1I 7.3.7 Intensities and Their Use in Band-Structure Determinations
pQk@
+r 7.3.8 Summary
u_6x{",5I 7.4 Experimental Band Structures
^<Zye>KO 7.4.1 One- and Two-Dimensional Systems
VJgYXPE
` 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
_z53r+A 7..4.3UPS Band Structures and XPS Density of States
98lz2d/Fcq 7.5 A Comment
ageTv/ References
N;*
wd< TiD|.a8S 8.Surface States, Surface Effects
.DHQJ|J-1 8.1 Theoretical Considerations
MGH2z: 8.2 Experimental Results on Surface States
z,(.` %h 8.3 Quantum-Well States
:i*
=s}cv 8.4 Surface Core-Level Shifts
5-POYug References
vAfYONU *V{Y.`\ 9.Inverse Photoelectron Spectroscopy
zG\:#,9 9.1 Surface States
K$5mDScoJ 9.2 Bulk Band Structures
i)7B :uA 9.3 Adsorbed Molecules
]r>m{"~E References
fzzk#jU hSG1f` 10. Spin-Polarized Photoelectron Spectroscopy
YFeL#)5y 10.1 General Description
LQJC ]*b1 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
jQdIeQD+ 10.3 Magnetic Dichroism
oq2-)F2/ References
^a=V. 8Od7e` 11. Photoelectron Diffraction
ISg-?h/ 11.1 Examples
C%AN4Mo 11.2 Substrate Photoelectron Diffraction
!nTI(-- 11.3 Adsorbate Photoelectron Diffraction
VUzRA"DP| 11.4 Fermi Surface Scans
bkiMF$K,K References
mLDuizWI ? s[!JeUA Appendix
BB.120v&N A.1 Table of Binding Energies
b
4A1M A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
[vOk= A.3 Compilation of Work Functions
YB376/ References
x57O.WdN Index